Publications Internationales

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    Predicting Methane Hydrate Formation Temperature in the Presence of Diverse Brines Using Explainable Artificial Intelligence
    (American Chemical Society, 2025) Nait Amar, Menad; Zeraibi, Noureddine; Alqahtani, Fahd Mohamad; Djema, Hakim; Benamara, Chahrazed; Saifi, Redha; Gareche, Mourad; Ghasemi, Mohammad; Merzoug, Ahmed
    Thisstudy presents three advanced techniques, includingthe leastsquares support vector machine (LSSVM), categorical boosting (CatBoost),and cascaded forward neural network (CFNN), to model methane hydrateformation temperature (MHFT) across various brines under a wide pressurerange. Utilizing a comprehensive data set of nearly 1000 samples,the models underwent rigorous training and testing phases. Graphicalanalyses and statistical assessment confirmed the high accuracy ofthe implemented models, with the CFNN scheme outperforming the others,achieving a total root-mean-square error (RMSE) of 0.3569 and an R2 of 0.9977. Comparison with existing modelsfurther highlighted the CFNN model’s superior performance.Additionally, the Shapley Additive exPlanning (SHAP) method was employedto enhance the aspects related to predictions’ explainabilityby assessing the impact of different inputs on the outcomes. Lastly,the proposed model holds significant potential for advancing industrialand academic applications related to hydrate phenomena
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    Modeling wax disappearance temperature using robust white-box machine learning
    (Elsevier Ltd, 2024) Nait Amar, Menad; Zeraibi, Noureddine; Benamara, Chahrazed; Djema, Hakim; Saifi, Redha; Gareche, Mourad
    Wax deposition is one of the major operational problems encountered in the upstream petroleum production system. The deposition of this undesirable scale can cause a variety of challenging problems. In order to avoid the latter, numerous parameters associated with the mechanism of wax deposition should be determined precisely. In this study, a new smart correlation was proposed for the accurate prediction of Wax disappearance temperature (WDT) using a robust explicit-based machine learning (ML) approach, namely gene expression programming (GEP). The correlation was developed using comprehensive experimental measurements. The obtained results revealed the promising degree of accuracy of the suggested GEP-based correlations. In this context, the newly-introduced correlations provided excellent statistical metrics (R2 = 0.9647 and AARD = 0.5963 %). Furthermore, performance of the developed correlation outperformed that of many existing approaches for predicting WDT. In addition, the trend analysis performed on the outcomes of the proposed GEP-based correlations divulged their physical validity and consistency. Lastly, the findings of this study provide a promising benefit, as the newly developed correlations can notably improve the adequate estimation of WDT, thus facilitating the simulation of wax deposition-related phenomena. In this context, the proposed correlations can supply the effective management of the production facilities and improvement of project economics since the provided correlation is a simple-to-use decision-making tool for production and chemical engineers engaged in the management of organic deposit-related issues.
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    Rheological and flow behavior of water-in-oil Pickering emulsions stabilized with organo-hectorite clay
    (Elsevier, 2021) Boutheina, Merad; Bekkour, Karim; Pierre, François; Gareche, Mourad
    The rheological and flow behaviors of Pickering emulsions are studied as a function of their water concentration. The studied emulsions are water-in-gasoil inverse emulsions stabilized with organo-hectorite clay. An in-line emulsion preparation was performed and a novel emulsification system was used. The emulsification system was tested and confirmed before performing pipe-flow measurements. A stress-controlled rheometer was used to study the rheological behavior of organoclay stabilized inverse emulsions. It was found that the emulsions exhibited a shear thinning with yield stress non-Newtonian rheological behavior and that the flow curves were well correlated using the Herschel-Bulkley model. Pressure loss and axial velocity measurements were studied to investigate the pipe-flow behavior of the emulsions. Axial velocity of the fluids was measured using an Ultrasonic Pulsed Doppler Velocimeter. It was shown that, up to 50 wt% water mass concentration, an exponential increase of yield stress and viscosity values is noticed, and the phase inversion point is not reached. In the range of the applied flow rates, turbulence took place only in the case of the lowest water cut (0 wt%). The Herschel-Bulkley rheological parameters were used to simulate the pipe-flow behavior of the studied fluids, and showed a satisfactory correlation with the in-line measurements. Furthermore, wall shear stress and velocity profiles were used to study the short-, medium-, and long-term stability of the emulsions
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    Rheological studies and optimization of Herschel–Bulkley parameters of an environmentally friendly drilling fluid using genetic algorithm
    (Springer, 2018) Ouaer, Hocine; Gareche, Mourad; Rooki, Reza
    The Herschel–Bulkley rheological parameters of an environmentally friendly drilling fluid formulated based on an Algerianbentonite and two polymers—hydroxyethyl cellulose and polyethylene glycol—have been optimized using a genetic algorithm.The effect of hydroxyethyl cellulose, temperature, pH and sodium chloride (NaCl) on the three-parameter Herschel-Bulkleymodel was also studied. The genetic algorithm technique provided improved rheological parameter characterization compared tothe nonlinear regression, especially in the case of drilling fluids formulated with sodium chloride making it a better choice.Furthermore, the oscillatory test offered more reliable yield stress values. The rheological parameters were found to be verysensitive to different conditions. Yield stress and consistency index increased with increasing the hydroxyethyl cellulose con-centration, reaching maximum at a temperature of 65 °C and decreased with decreasing pH and also when adding sodiumchloride to the drilling fluid. The flow index changed inversely to yield stress and consistency index. The physical origins of thesechanges in rheological parameters were discussed and correlation between variation in rheological parameters and bentonitesuspension properties were concluded. Based on these results, it is recommended to use the proposed formulation of drilling fluidat high temperature and when the formation of alkaline pH is encountered due to the gelation mechanism and to select theoptimum concentration of NaCl to avoid degradation of the rheological parameters
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    Thermal gelation of partially hydrolysed polyacrylamide/polyethylenimine mixtures using design of experiments approach
    (Elsevier, 2019) Ghriga, Mohammed Abdelfetah; Hasanzadeh, Mahdi; Gareche, Mourad; Lebouachera, Seif El Islam; Drouiche, Nadjib; Grassl, Bruno
    Polyethylenimine crosslinked polymer gels are gaining a huge interest in conformance control applications in oilfields. They are used to reduce the production of undesirable fluids (water & gas) by blocking the fractures that connect injection and production wells. In this paper, a statistical analysis on the thermal gelation of well characterized reactants namely partially hydrolysed polyacrylamide (PHPA) (Mw = 5.1 million Daltons and hydrolysis degree = 6%) and polyethylenimine (PEI) (Mw = 19.2 kilo Daltons and branching degree = 59%), was conducted using response surface methodology (RSM). A four factor doehlert matrix was employed in designing the experiments and evaluating the gelation time as function of salinity (0–8 g/L NaCl), polymer (PHPA) and crosslinker (PEI) concentrations, temperature (70 °C–90 °C) and their corresponding combinations. As a result, the gelation time was found to strongly vary with salinity, temperature and PHPA concentration following a nonlinear mathematical model. The analysis of variance (ANOVA) of this model revealed its significance in a 95% confidence level against experimental data. In a second part, an experimental investigation was carried out to understand the interaction between PHPA and PEI. To do so, the viscosity variations of analogue mixtures prepared with low molecular weight (Mw) polymers, such as polyacrylamide (PAM) and polyacrylic acid (PAA), were monitored using capillary viscometry at different conditions of temperature, pH and reaction time. The PAM/PEI mixtures showed a remarkable viscosity increase at typical pH of around 10 when cured at 80 °C. While, the PAA/PEI mixtures underwent precipitation at pH of around 6 revealing the strong interaction between PAA and PEI at this condition
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    Review of recent advances in polyethylenimine crosslinked polymer gels used for conformance control applications
    (Springer, 2019) Ghriga, Mohammed Abdelfetah; Grassl, Bruno; Gareche, Mourad; Khodja, Mohamed; Lebouachera, Seif El Islam; Andreu, Nathalie; Drouiche, Nadjib
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    Relationship between the fractal structure with the shear complex modulus of montmorillonite suspensions
    (Elsevier, 2016) Gareche, Mourad; Allal, A.; Zeraibi, Noureddine; Roby, F.; Azril, N.; Saoudi, L.
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    Numerical study of a thermodependent non-Newtonian fluid flow between vertical concentric cylinders
    (Elsevier, 2007) Zeraibi, Noureddine; Amoura, M.; Benzaou, A.; Gareche, Mourad
    In this paper, we present a numerical investigation of the thermal convection for a thermodependent non-Newtonian fluid in an annular space between two coaxial rotating cylinders. The rheological behaviour of the fluid can be expressed through the Ostwald-De-Waele power law: View the MathML sourceτ=Kγ˙n; all fluid properties except consistency index K are constant. K–T relation used is K = K0e−bT. The problem is studied when the heated inner cylinder is rotating around the common axis with constant angular velocity and the cooled outer cylinder is at the rest. The horizontal endplates are assumed adiabatic. The governing equations are solved using mixed finite elements method. The influence of the temperature on the structure of the dynamic and thermal fields is examined
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    Modélisation du module complexe de cisaillement des suspensions de bentonite = Modelling of complex shear modulus of bentonite suspensions
    (Groupe français de rhéologie, Sophia Antipolis, FRANCE, 2009) Allal, A.; Gareche, Mourad; Dupin, J. C.; Roby, F.; Zeraibi, Noureddine
    Dans ce travail, nous avons étudié le comportement rhéologique de suspensions de bentonite pour diverses concentrations massiques (2, 4, 5, 6 et 8 %). Nous nous sommes intéressés plus particulièrement à la viscoélasticité linéaire, avec pour objectif de faire le lien entre la structure fractale des ces suspensions et le module de cisaillement complexe. A partir de la dimension fractale des gels formés par les particules d'argile en interaction dans les suspensions de bentonite, nous avons modélisé la variation de leurs modules complexes de cisaillement en fonction de la fréquence